LLM Summaries - vdW materials

We present an infrared spectroscopy study of the layered topological semimetal TaNiTe$_5$, a material with a quasi-one-dimensional structure and strong in-plane anisotropy. Despite its structural features, infrared reflectivity and electronic transport measurements along the $a$ and $c$ crystallographic axes show metallic behavior without evidence of reduced dimensionality. Optical conductivity reveals an anisotropic but conventional metallic response with low scattering rates and a single sharp infrared-active phonon mode at $396$ cm$^{-1}$ ($49$ meV). Ab initio calculations closely match the experimental optical data and confirm a three-dimensional electronic structure. Our results demonstrate that TaNiTe$_5$ behaves as a three-dimensional anisotropic semimetal in its electronic and optical properties.

Electric conductivities may reveal the topological and magnetic properties of band structures in solids, especially for two-dimensional unpaired Dirac fermions. In this work, we evaluate the longitudinal and Hall conductivity for unpaired Dirac fermions in the framework of the self-consistent Born approximation and find a nearly semi-elliptic relation between the minimal conductivity and Hall conductivities in the Dirac fermions. Near the charge neutrality point, disorder may drive a metal-insulator transition, and enhance the longitudinal conductivity. For the massless case, the minimal conductivity $\sigma_{xx}^*$ coexists with the half-quantized Hall conductivity $e^2/2h$, forming an indicator for the parity anomalous semimetal. The relation signals a disorder-induced metallic phase that bridges two topologically distinct insulating phases, and agrees with the recent experimental observation in magnetic topological insulators.

We study two-dimensional Dirac fermions in a one-dimensional mass superlattice under a perpendicular magnetic field. Using exact solutions for isolated and finite arrays of domain walls, we demonstrate the persistence of Jackiw-Rebbi modes with a field-dependent renormalized velocity. For the periodic case, we adopt a gauge-invariant projection method onto magnetic Bloch states, valid for arbitrary fields and mass profiles, which yields dispersive Landau levels, and confirm its accuracy by comparison with finite arrays spectra. From the miniband spectra we predict modified quantum Hall plateaus and Weiss-like magnetoconductivity oscillations, characterized by a strongly reduced amplitude and a $\pi/2$ phase shift compared to electrostatic superlattices.

Nanoscale topologically non-trivial magnetization configurations generate significant interest due to both the fundamental properties of their knotted structures and their potential applications in ultra-efficient computing devices. While such textures have been widely studied in two dimensions, three-dimensional (3D) systems can yield more complex configurations, resulting in richer topologies and dynamic behaviors. However, reliably nucleating these 3D textures has proven challenging, and so far, 3D configurations such as vortex rings and hopfions can often only be observed forming spontaneously in relatively uncontrolled manners. Here, we demonstrate that through the 3D nanopatterning of chiral single crystal helimagnets into nano-tori, the controlled formation of a magnetic double helix can be achieved. This surface-localized topological state is stabilized by the interplay of intrinsic exchange interactions of the single crystal with the extrinsic emergent effects of the patterned geometry. These double helices host magnetic defects akin to supercoiling in circular DNA and climbing vines. We expect this study to serve as a foundation for future research combining single crystal systems with 3D nanopatterning, offering a new degree of control over emergent phenomena in nanoscale magnets and wider quantum material systems.

The discovery of high-temperature superconductivity in hydrogen-rich compounds under extreme pressures has prompted great excitement, intense research, but also debate over the past decade. Electrical transport has been the primary diagnostic tool for identifying superconductivity in these systems, whereas complementary probes, including magnetic, spectroscopic, tunnelling and ultrafast methods, remain mostly qualitative due to experimental constraints and sample heterogeneity. Recent concerns over their reliability have fuelled controversy, leading to scepticism and pointing out the need for alternative, quantitative approaches. In this study, we acquired unprecedented high-quality Raman spectra of hexagonal LaH10 at approximately 145 GPa and low temperatures, in conjunction with electrical transport measurements. Upon cooling, we observe a drop of resistivity and simultaneous remarkable variations of phonon frequencies and linewidths. These effects are interpreted and perfectly reproduced by the Migdal-Eliashberg theory, providing a definitive proof of phonon-mediated superconductivity and enabling a quantitative determination of the superconducting energy gap. Our results establish Raman spectroscopy as a robust, contact-free probe with micrometric resolution for studying high temperature superconductivity, opening a powerful route to its discovery and characterization.

We derive the full spectrum of decorated Cayley trees that constitute tree analogs of selected two-dimensional Euclidean lattices; namely of the Lieb, the double Lieb, the kagome, and the star lattice. The common feature of these Euclidean lattices is that their nearest-neighbor models give rise to flat energy bands interpretable through compact localized states. We find that the tree analogs exhibit similar flat or nearly flat energy bands at the corresponding energies. Interestingly, such flat bands in the decorated Cayley trees acquire an interpretation that is absent in their Euclidean counterparts: as edge states localized to the inner or the outer boundary of the tree branches. In particular, we establish an exact correspondence between the Lieb-Cayley tree and an ensemble of one-dimensional Su-Schrieffer-Heeger chains, which maps topological edge states on one side of the chains to flat-band states localized in the bulk of the tree, furnishing the flat energy band with a topological stability. Similar mapping to topological edge states or to states bound to edge defects in one-dimensional chains is shown for flat-band states in all the considered tree decorations. We finally show that the persistence of exact flat bands on infinite decorated trees (i.e., Bethe lattices) arises naturally from a covering interpretation of tree graphs. Our findings reveal a rich landscape of flat-band and topological phenomena in non-Euclidean systems, where geometry alone can generate and stabilize unconventional quantum states.

We report a comprehensive investigation of the quasi-one-dimensional spin-chain compound Ca3CoIrO6 (CCIO) using a combination of structural, magnetic, thermodynamic, transport, Raman, and dielectric measurements. Temperature-dependent neutron powder diffraction confirms the rhombohedral R-3c structure down to 5 K without any structural phase transition. DC magnetization, ac susceptibility, and relaxation measurements reveal a gradual evolution from a high-temperature paramagnetic-like state to a partially disordered antiferromagnetic (PDA) state below 100 K, accompanied by slow cluster-like spin dynamics followed by a freezing transition near 30 K. Isothermal magnetic hysteresis M(H) loops demonstrate partial chain freezing, while robust exchange bias is observed in field-cooled protocols, highlighting the interplay between PDA ordering and frozen spins. Resistivity and specific heat data indicate strong coupling between spin and charge degrees of freedom, accompanied by activated transport behavior. Raman spectroscopy identifies pronounced anomalies in phonon frequencies and linewidths across multiple magnetic regimes, reflecting strong spin-lattice coupling. Polarization-electric field (P-E) measurements reveal temperature-dependent crossovers from linear dielectric to weakly hysteretic behavior, consistent with short-range polar correlations driven by spin-lattice interactions. These findings establish CCIO as a prototypical quasi-one-dimensional frustrated spin-chain system where geometric frustration, spin-orbit coupling, and low-dimensionality generate field-tunable PDA order, glassy spin dynamics, exchange bias, and magnetodielectric coupling. These results provide new insights into frustration-driven phases in low-dimensional oxides and point towards potential multifunctional applications based on intrinsic magnetodielectric and exchange bias phenomena.

We consider hairy, magnetic black brane solutions to Einstein-Maxwell-Chern-Simons-Dilaton theory with full back-reaction of the scalar and gauge fields and compute the time evolution with time dependent sources. The dual field theory's 't Hooft anomaly leads to long-lived current oscillations in the low temperature limit long after the electric pulse which created these modes has been switched off. We find that, generally, non-linear effects increase the decay rates of long-lived modes by a temperature dependent amount. Nonetheless, our results suggest that the life-time of time-translation symmetry breaking states can be made arbitrarily large if the temperature after the quench is sufficiently small. Experimentally this might be realizable in Weyl semimetals.

Resonant parametric modulation is a major tool of studying magnetic systems. For a spin-1/2 chain in a strong magnetic field, the resulting excitations can be mapped on fermionic excitations in the Kitaev chain. We show that the response to the modulation turn-on allows one to reveal dynamical aspects of the nontrivial topology of the periodic chain. In the topological regime, depending on how fast the turn-on is, the system displays the absence of spatial magnetization correlations or their increase with the increasing detuning of the modulation from resonance. The transition between the topological and trivial regimes is controlled by the modulation frequency.

Hydrodynamic interactions can generate rich emergent structures in active matter systems. Using large-scale hydrodynamic simulations, we demonstrate that hydrodynamic coupling alone can drive spontaneous self-organization across a hierarchy of spatial and temporal scales in confined suspensions of torque-driven particles at moderate Reynolds numbers. Spinners first self-assemble into dimers, which crystallize into a hexatic lattice and subsequently undergo a collective tilting instability. The resulting tilted dimers rotate and synchronize through hydrodynamic repulsion, which can be tuned by the Reynolds number. Upon synchronization, the polar director develops splay and bend deformations and nucleates topological defects with charges of $\pm1$. These defects induce long-wavelength concentration gradients and drive crystal vortex dynamics spanning hundreds of particle diameters. Our results reveal a purely hydrodynamic route to synchronization and defect-mediated dynamics in chiral active matter, without explicit alignment rules or interparticle forces.

We propose a microscopic, weak-coupling mechanism by which generic Chern bands relax toward ideal bands. We consider coupling interacting electrons to a Caldeira-Leggett like Ohmic bosonic bath. Using the Born-Markov approximation, Slater determinant states of a Chern band under Hartree-Fock approximation evolve toward Slater determinant states corresponding to an ideal Chern band. We validate our proposal by performing numerical simulation of a massive Dirac model, showing that the Berry curvature and quantum metric indeed co-evolve to saturate the trace condition. Our proposal provides a concrete dissipative route to realize ideal Chern bands, a fundamental building block for the stabilization of fractional Chern insulators.

It is known that, under appropriate conditions, mean-field interactions can be canceled in binary BEC, leading to the formation of the Lee-Huang-Yang (LHY) superfluid, in which the nonlinearity is solely represented by the quartic LHY term. In this work we systematically investigate the existence, stability and evolution of hopfion states in this species of quantum matter. They are characterized by two independent topological winding numbers: inner twist $s$ of the vortex-ring core and overall vorticity $m$. The interplay between the LHY self-repulsion and a trapping harmonic-oscillator potential results in stability of the hopfions with $s = 1$ and $m$ ranging from $0$ to $4$. The hopfions exhibit distinct topological phase distributions along the vertical axis and the radial direction in the horizontal plane. Their effective radius and peak density increase with the chemical potential, along with expansion of the vortex-ring core. Although the instability domain of the hopfion modes broadens with the increase of $m$, stable hopfions persist in a wide range of the chemical potential, up to $m=4$, at least, provided that the norm exceeds a certain threshold value. The predictions are experimentally accessible in currently used BEC setups.

arXiv:2505.15521v2 Announce Type: replace-cross Abstract: One of premier utilities of present day noisy quantum computers is simulation of many-body quantum systems. We study how long in time is such a discrete-time simulation representative of a continuous time Hamiltonian evolution, namely, a finite time-step introduces so-called Trotterization errors. We show that the truncated operator propagator (Ruelle-Pollicott resonances) is a powerful tool to that end, as well as to study prethermalization and discrete time crystals, including finding those phenomena at large gate duration. We show that the effective energy is more stable than suggested by Trotter errors -- a manifestation of prethermalization -- while all other observables are not. Even the most stable observable though deteriorates in the thermodynamic limit. Different than in classical systems with the strongest chaos, where the faithfulness time (the shadowing time) can be infinite, in quantum many-body chaotic systems it is finite. A corollary of our results is also that, opposite to previous claims, there is no Trotterization transition in non-integrable many-body quantum systems. We demonstrate our results on a one-dimensional (1d) kicked Ising model, as well as on 1d kicked XX model and 2d kicked Ising model. The truncated propagator is also used to calculate the energy diffusion constant in the tilted-field Ising model with high accuracy.

We study topological insulators under dephasing noise. With examples of both a $2d$ Chern insulator and a $3d$ topological insulator protected by time-reversal symmetry, we demonstrate that there is a phase transition at finite dephasing strength between phases with nontrivial and trivial topological indices. Here the topological index is defined through the correlation matrix. The transition can be diagnosed through the spectrum of the whole correlation matrix or of a local subsystem. Interestingly, even if the topological insulator is very close to the topological-trivial critical point in its Hamiltonian, it still takes finite strength of dephasing to change the topological index, suggesting the robustness of topological insulators under dephasing. We further consider Chern insulators in the presence of real-space disorder, which exhibit a ground-state transition between topological and Anderson insulating phases. We find that even strongly-disordered Chern insulators, close to the critical disorder strength, exhibit robustness with respect to dephasing.

The potential of solid-state quantum emitters for applications critically depends on several key figures of merit. One of the most important is the quantum coherence of the emitted single photons, which can be compromised by fast dephasing and spectral diffusion. In hexagonal boron nitride (hBN), blue-emitting color centers (or B centers) are seen as favorable in this regard, in the light of prior studies mainly based on resonant excitation. Yet, their coherence properties in the more accessible regime of non-resonant excitation (or photoluminescence) has not been extensively characterized. Here, we investigate the coherence and spectral diffusion of the photoluminescence from a B center in the continuous wave regime using photon correlation Fourier spectroscopy. We determine that the emission lineshape consists in a homogeneous contribution, whose linewidth increases with the laser power, and which is broadened by spectral diffusion at a timescale of 10 to 100 microseconds. At low power and short time, the emission line is only a factor ~2 above the Fourier limit, while at long times, the inhomogeneous linewidth increases up to more than a gigahertz. Our work deepens the understanding of decoherence processes of this preeminent family of quantum emitters in hBN.

Autonomous laboratories typically rely on data-driven decision-making, occasionally with human-in-the-loop oversight to inject domain expertise. Fully leveraging AI agents, however, requires tightly coupled, collaborative workflows spanning hypothesis generation, experimental planning, execution, and interpretation. To address this, we develop and deploy a human-AI collaborative (HAIC) workflow that integrates large language models for hypothesis generation and analysis, with collaborative policy updates driving autonomous pulsed laser deposition (PLD) experiments for remote epitaxy of BaTiO$_3$/graphene. HAIC accelerated the hypothesis formation and experimental design and efficiently mapped the growth space to graphene-damage. In situ Raman spectroscopy reveals that chemistry drives degradation while the highest energy plume components seed defects, identifying a low-O$_2$ pressure low-temperature synthesis window that preserves graphene but is incompatible with optimal BaTiO$_3$ growth. Thus, we show a two-step Ar/O$_2$ deposition is required to exfoliate ferroelectric BaTiO$_3$ while maintaining a monolayer graphene interlayer. HAIC stages human insight with AI reasoning between autonomous batches to drive rapid scientific progress, providing an evolution to many existing human-in-the-loop autonomous workflows.

Most engineered pilings require substantially more force to be driven into the ground than they can resist during extraction. This requires relatively heavy equipment for insertion, which is problematic for anchoring in hard-to-access sites, including in extraterrestrial locations. In contrast, for tree roots, the external reaction force required to extract is much greater than required to insert--little more than the weight of the seed initiates insertion. This is partly due to the mechanism by which roots insert into the ground: tip extension. Proof-of-concept robotic prototypes have shown the benefits of using this mechanism, but a rigorous understanding of the underlying granular mechanics and how they inform the design of a robotic anchor is lacking. Here, we study the terradynamics of tip-extending anchors compared to traditional piling-like intruders, develop a set of design insights, and apply these to create a deployable robotic anchor. Specifically, we identify that to increase an anchor's ratio of extraction force to insertion force, it should: (i) extend beyond a critical depth; (ii) include hair-like protrusions; (iii) extend near-vertically, and (iv) incorporate multiple smaller anchors rather than a single large anchor. Synthesizing these insights, we developed a lightweight, soft robotic, root-inspired anchoring device that inserts into the ground with a reaction force less than its weight. We demonstrate that the 300 g device can deploy a series of temperature sensors 45 cm deep into loose Martian regolith simulant while anchoring with an average of 120 N, resulting in an anchoring-to-weight ratio of 40:1.

In this paper we attempt to construct the topological theory of superfluid helium $4$ in the framework of the (rigid) $U(1)$ model in which the initial $U(1)$ group is destroyed with appearance of (topologically nontrivial) domains separated by domain walls treated as step voltages between domains (e.g. with neighboring topological numbers). This can explain the superfluid properties in a helium $4$ specimen as well as the appearance of topologically nontrivial vortices therein.

The non-Hermitian skin effect (NHSE), characterized by the extensive localization of bulk modes at the boundaries, has attracted significant attention as a hallmark feature of non-Hermitian topology. This localization invalidates the conventional Bloch band theory, necessitating an analysis under open boundary conditions even in the thermodynamic limit. The Amoeba formulation addresses this challenge by computing the spectral potential rather than the spectrum itself. Based on the (strong) Szeg\"o limit theorem and its topological generalization, this approach reduces the evaluation of the potential to an optimization problem involving the Ronkin function. However, while the generalized Szeg\"o limit theorem is formally applicable in arbitrary dimensions, its implementation is limited to single-band systems, and its applicability to multiband systems remains unclear. In this paper, we establish the Wiener-Hopf factorization (WHF) of the non-Bloch Hamiltonian as a powerful framework, providing a unified and rigorous foundation for Amoeba analysis in multiband systems. By combining the WHF with Hermitian doubling, we first elucidate the applicability criteria for the generalized Szeg\"o limit theorem in multiband systems. We then show that the WHF provides the natural mathematical origin for the symmetry-decomposed Ronkin function in symmetry class AII$^\dagger$, leading to a rigorous proof of the generalized Szeg\"o limit theorem for these systems and opening a path toward systematic generalizations to other symmetry classes.

We introduce an infinite, scale-aligned hierarchy of one-dimensional, frustration-free Hamiltonians by forbidding the minimal forbidden factors of the Fibonacci word up to length $F_K$, the $K$-th Fibonacci number. The ground-state languages have exponential growth constants $\lambda_K$ that decrease monotonically, starting from the value associated with the ``golden chain'' (approximately 1.618) and progressing toward 1. This process yields a staircase of topological-entropy plateaus that flows to an aperiodic fixed point, also known as the Fibonacci subshift. The first nontrivial rung ($K=4$) is the ``Plastic chain,'' which forbids \texttt{SS} and \texttt{LLL}. We prove its ground-state counts follow a specific four-term linear recurrence relation and provide a closed-form solution governed by the plastic constant $\rho\approx 1.3247$. We propose an energy-entropy scaling where the energy penalty for each new forbidden pattern is proportional to the logarithmic ratio of the growth constants from the previous and current rungs, turning the sequence of projectors into an explicit renormalization-group flow from the initial high-entropy phase to the zero-entropy aperiodic fixed point. Algebraically, exact Temperley-Lieb braiding compatibility holds only at the base rung, $K=3$ (which forbids only \texttt{SS}); higher rungs define constrained aperiodic Hamiltonian codes rather than Temperley-Lieb representations. Small instances realized on a D-Wave quantum annealer match these predictions: $K=3$ is trivial, $K=4$ resolves a unit gap with moderate success, and $K\ge 5$ instances require reverse annealing to exceed $99\%$ success, clarifying reduction penalties and embedding variability.

We study conformal field theories (CFTs) and their classifications from a modern perspective based on the abstract algebraic formalism of symmetries or conserved charges, known as symmetry topological field theories (SymTFTs). By studying the algebraic structure of the SymTFTs in detail, we found a natural generalization of the quantum dimensions associated with (pseudo-)Hermitian systems and (non)-unitary CFTs. These generalized data of SymTFTs provide classifications of massless and massive renormalization group flows, which will describe the quantum phase transitions of the corresponding pseudo-Hermitian systems. Moreover, our discussions straightforwardly enable one to relate a general class of coset constructions or level-rank dualities to domain wall problems between topological quantum field theories (or a series of corresponding quantum phase transitions related to the Higgs mechanism). Our work provides a systematic reduction and classification of algebraic data, symmetries, for pseudo-Hermitian systems based on ideas from established mathematical fields, linear algebra and ring theory.