Moir\'e flat bands in rhombohedral multilayer graphene provide a platform for exploring interaction-driven topological phases, where a single isolated band often forms a Chern band. However, non-Abelian degenerate Chern bands with internal symmetries such as $\mathrm{SU}(N)$ have so far been realized only in highly engineered systems. Here, we show that a doubly degenerate non-Abelian Chern band with Chern number $|C|=1$ emerges spontaneously at filling $\nu=2$ in rhombohedral 3-, 4-, and 5-layer graphene, regardless of the presence of an hBN substrate. Using self-consistent Hartree-Fock calculations, we map out phase diagrams as functions of displacement field and electronic periodicity, and analytically demonstrate that the Fock term drives spontaneous symmetry breaking and generates non-Abelian Berry curvature. We further show that this non-Abelian topology is characterized by $\mathrm{SU}(2)$ gauge flux threading the noncontractible cycles of the Brillouin zone, leading to a global non-Abelian holonomy. Our findings unveil a new class of interaction-driven non-Abelian topological phases, distinct from quantum anomalous Hall and fractional Chern phases.
Nature Nanotechnology, Published online: 15 April 2026; doi:10.1038/s41565-026-02149-6
Printed MoS2 memristive networks yield spiking neurons with multi-order complexity. Thermally activated snap-back produces physiological waveforms that stimulate mouse Purkinje neurons, offering a scalable platform for bio-realistic neuromorphic hardware and brain–machine interfaces.Copper‐graphene composite (CGC) conductors are widely considered as a potential alternative to pure copper (Cu). Yet, the effect of graphene (Gr) on the electrical conductivity of CGCs remains elusive, and their electrical performance is still controversial. This work addresses these unresolved questions by unambiguously quantifying how the electrical properties of CGCs depend on the characteristics of Gr and Cu. Gr is synthesized on Cu foils, foams, and wires by utilizing a wide range of chemical vapor deposition conditions to independently control their characteristics. Then the Gr‐enhanced electrical conductivity (Δσ) is characterized for CGCs with different Cu geometries and Gr qualities. This study confirms that unprecedented electrical conductivity (Δσ = 17.1%) can be achieved only when both Gr and Cu are carefully optimized. Specifically, the study reveals three key factors: (1) Δσ is positively correlated with continuity of Gr; (2) CGCs with a continuous monolayer Gr exhibit a strong Δσ − A s linear relation where A s is the specific surface area of a CGC; and (3) Δσ becomes more pronounced when a Cu matrix has a curved cross‐section. This work reveals the fundamental mechanisms of how Gr influences the overall electrical conductivity of CGCs and, therefore, is a crucial step toward designing and manufacturing high‐performance CGC conductors for emerging applications.
Van der Waals (vdW) heterostructures enable tailored electronic and magnetic phases by stacking atomically thin layers with pristine interfaces. Here, we investigate fully 2D Cr2Ge2Te6/WTe2 heterostructures and identify a strong enhancement of ferromagnetism in Cr2Ge2Te6 (CGT). Magnetotransport measurements across multiple devices with WTe2 thicknesses ranging from monolayer to bulk reveal a robust anomalous Hall effect together with a more than two fold increase of the Curie temperature and substantially enhanced coercive fields. Interface microscopy confirms chemically abrupt vdW interfaces with no detectable interdiffusion, while control experiments rule out processing- or stray-field-induced artifacts. Our experiments and theoretical calculations demonstrate that interfacial charge transfer renders CGT conductive and that proximity-induced lattice distortions in CGT enhance exchange and magnetocrystalline anisotropy. These results establish strain-mediated lattice reconstruction as a strategy for engineering high-temperature magnetic order in 2D heterostructures and clarify that modifications within the magnetic layer itself can govern proximity effects in vdW stacks.
Van der Waals (vdW) heterostructures enable tailored electronic and magnetic phases by stacking atomically thin layers with pristine interfaces. Here, we investigate fully 2D Cr2Ge2Te6/WTe2 heterostructures and identify a strong enhancement of ferromagnetism in Cr2Ge2Te6 (CGT). Magnetotransport measurements across multiple devices with WTe2 thicknesses ranging from monolayer to bulk reveal a robust anomalous Hall effect together with a more than twofold increase of the Curie temperature and substantially enhanced coercive fields. Interface microscopy confirms chemically abrupt vdW interfaces with no detectable interdiffusion, while control experiments rule out processing- or stray-field-induced artifacts. Our experiments and theoretical calculations demonstrate that interfacial charge transfer renders CGT conductive and that proximity-induced lattice distortions in CGT enhance exchange and magnetocrystalline anisotropy. These results establish strain-mediated lattice reconstruction as a strategy for engineering high-temperature magnetic order in 2D heterostructures and clarify that modifications within the magnetic layer itself can govern proximity effects in vdW stacks.
Van der Waals heterostructures made from atomically thin transition metal dichalcogenides (TMD) and graphene have emerged as a building block for optoelectronic devices. Such systems are also uniquely poised to investigate interfacial coupling as well as photoinduced charge and energy transfer in the 2D limit. Recent works have revealed efficient photoluminescence quenching and picosecond transfer in TMD/graphene heterostructures. However, key questions regarding the transfer mechanisms remain. Here, employing time-resolved photoluminescence spectroscopy with 1~ps resolution in MoSe$_2$ monolayer directly coupled to a few-layer ``staircase-like'' graphene flake, we consistently observe an exciton transfer time of $\approx 2.5~\mathrm{ps}$ at cryogenic temperature that is marginally affected by the number of graphene layers. Remarkably, exciton transfer vanishes in samples consisting in an MoSe$_2$ monolayer separated from graphene by a thin dielectric spacer of hexagonal boron nitride, as soon as the spacer thickness reaches 1~nm. These results suggest that charge tunnelling processes govern exciton dynamics. Other mechanisms mediated the dipolar interactions (F\"orster-type energy transfer) have no measurable impact on bright excitons (with near-zero center of mass momentum) but may accelerate the relaxation of finite momentum ``hot'' excitons, leading to larger photoluminescence quenching than anticipated based on the measurements of the photoluminescence decay rates. Our work provides important insights into charge and energy transfer in van der Waals materials with direct implications for energy harvesting and funneling.
2D Janus structures break the mirror symmetry, thereby leading to the emergence of novel properties. Anion‐ordered Janus structures hold potential for developing large spontaneous polarization ferroelectrics. However, van der Waals disordered alloys are generally more thermodynamically stable; anion‐ordered Janus structures can only be realized in certain monolayer transition metal dichalcogenides so far. The polarization in these materials cannot be reversed; therefore, the realization of anion order triggered ferroelectricity remains a challenge. Here, we report that S/Se ordering induces Janus ferroelectricity in SnS 0.6 Se 0.4 nanobelts with a high Curie temperature of approximately 600 K. The second‐harmonic generation of SnS 0.6 Se 0.4 nanobelts is approximately 300 times more intense than that of SnS nanobelts. The switchable spontaneous polarization of SnS 0.6 Se 0.4 nanobelts was confirmed by piezoelectric force microscopy, representing the first realization of anion‐ordered Janus ferroelectricity. This anion ordering induces a structural phase transition from the non‐ferroelectric Pnma to the ferroelectric phase Pm. Our work has realized a periodically anion‐ordered Janus structure with ferroelectricity in van der Waals materials and provided a candidate material for novel non‐volatile memory devices and optoelectronic applications.
Twist-engineering of topological phases in two-dimensional materials offers a powerful route to modulate electronic structure beyond conventional strain or chemical control. In particular, group 15 (pnictogens) monolayers such as bismuthene provide an ideal platform due to their strong intrinsic spin-orbit coupling (SOC) and robust topological character. Here, we investigate a previously unexplored heterostructure consisting of a $\beta$-bismuthene monolayer rotated by 30$^\circ$ on a planar bismuthene layer stabilized on a SiC(0001) substrate. Using first-principles calculations, we demonstrate that this specific rotational alignment induces a unique interlayer orbital hybridization which, combined with the strong SOC and the naturally broken inversion symmetry, gives rise to a pronounced Rashba spin-splitting, absent in the isolated monolayers. The topological nature of the system is confirmed through the calculation of the Z2 topological invariant and Spin Hall Conductivity (SHC), revealing a robust Quantum Spin Hall (QSH) phase with an enhanced topological response compared to the individual layers. Furthermore, we explore the chemical tunability of this system via Sb substitution, showing that the gradual reduction of SOC systematically narrows the band gap while preserving the non-trivial topology. Our results establish large-angle twisted group 15 heterostructures as a versatile platform for engineering spin-orbit-driven phenomena and advancing topological spintronics.
Magnetic skyrmions and higher-order topological spin textures offer rich opportunities for multi-level information encoding, yet their deterministic stabilization and transformation under geometric confinement at room temperature remain poorly understood. Here, we demonstrate that geometric confinement acts as a robust and universal control parameter that governs a hierarchical transformation pathway of chiral spin textures in Pt/Co/W multilayer micro-tracks. As the confinement increases, extended labyrinth domains fragment into isolated skyrmions, followed by the systematic suppression of skyrmion pairs and the preferential stabilization of compact higher-order textures. We find that confinement strongly enhances the formation of skyrmioniums via recombination and promotes their subsequent evolution into uniform skyrmion bags by capturing additional skyrmions. Statistical analysis reveals a confinement-driven redistribution of topological populations, with skyrmion bags emerging as the dominant state in the narrowest tracks. Supported by micromagnetic simulations, our results establish geometric confinement as a deterministic selector of complex topological textures and reveal a previously unexplored route for engineering higher-order skyrmionic states at room temperature. These findings provide a scalable materials strategy for multistate skyrmion-based spintronic and memory architectures.
Author(s): Sen Shao, Wei-Chi Chiu, Tao Hou, Naizhou Wang, Ilya Belopolski, Yilin Zhao, Jinyang Ni, Qi Zhang, Yongkai Li, Jinjin Liu, Mohammad Yahyavi, Yuanjun Jin, Qiange Feng, Peiyuan Cui, Cheng-Long Zhang, Yugui Yao, Zhiwei Wang, Jia-Xin Yin, Su-Yang Xu, Qiong Ma, Wei-bo Gao, Md Shafayat Hossain, Arun Bansil, and Guoqing Chang
Chiral charge density waves (CDWs) have attracted intense interest due to their exotic quantum properties, yet the microscopic origin of structural chirality emerging from correlated charge order remains elusive. Here, we reveal that the interlayer phases of CDW vectors, an overlooked degree of free…
[Phys. Rev. Lett. 136, 156101] Published Tue Apr 14, 2026
Topologically nontrivial magnetic textures such as skyrmions offer promising opportunities for spintronic applications. In recent years, it has been shown that the magnetic properties of layered materials can be affected by depositing chiral molecules on the surface, while the influence of chiral overlayers on skyrmion properties such as their stability and interactions remains largely unexplored. To address this challenge, we employ wide-field nitrogen-vacancy (NV) magnetometry to directly image skyrmions in chiral-molecule-functionalized magnetic thin films, enabling quantitative mapping of magnetic stray fields over extended areas under ambient conditions. Using pixel-resolved optically detected magnetic resonance (ODMR) combined with controlled magnetic fields, we reproducibly nucleate and probe skyrmion states in CoFeB ferromagnetic samples, enabling quantitative investigation of their properties. We find evidence for enantioselective and magnetic-field-polarity-dependent modifications of skyrmion diameter, spacing, and shape, pointing to a possibility of molecular control of topological spin textures via magneto-chiral coupling.
Non-Hermitian band descriptions capture how loss, gain, and environmental coupling reshape quantum matter, yet most experimental tests rely on wave-based or dynamical probes. Here we establish a new equilibrium route to exceptional physics in Dirac materials: in the weakly non-Hermitian regime, the thermodynamic density of states and the quantum capacitance exhibit a universal equilibrium approach to the exceptional point. In our minimal non-reciprocal graphene model, the hopping imbalance reduces the Dirac velocity as $v_F=v\sqrt{1-\beta^2}$, implying that the low-energy density of states, the thermodynamic density of states, and the quantum capacitance all scale as $(1-\beta^2)^{-1}$ as $|\beta|\to 1^-$. Consequently, at charge neutrality the quantum capacitance remains linear in temperature but with a diverging prefactor, while the inverse response softens linearly on approaching the exceptional point. In a magnetic field, this manifests as a collapse of the Landau-level spacing and a corresponding crowding of thermally active levels. Complementarily, the biorthogonal Bloch states exhibit a Petermann factor $K=(1-\beta^2)^{-1}$, which isolates the irreducibly non-Hermitian effect of eigenvector non-orthogonality. These results identify quantum capacitance as an experimentally accessible bulk equilibrium probe of effective non-Hermiticity in Dirac materials.
We show that electron drag by nonequilibrium phonons describes the actual waveform and spectrum of terahertz pulses generated during femtosecond laser irradiation of metals. In contrast to previous models, there is a picosecond delay in the drag force development due to the relatively slow lattice heating and finite phonon lifetime. We also predict that, at high pump fluences, a macroscopic deformation wave enhances nonlinearly the drag force and terahertz response. Our results establish the terahertz pulse waveform as a direct probe of ultrafast lattice dynamics in metals.
The coexistence of topological states with different dimensionalities in a single crystalline system offers a unique platform to study the interplay of distinct fermionic excitations. Here, integrating first-principles calculations with symmetry analysis, we propose the three-dimensional boron allotrope $P6_3$-$\text{B}_{30}$ as an ideal, structurally stable candidate for exploring multidimensional topological physics. Benefiting from the practically negligible spin-orbit coupling of the light-element framework, $P6_3$-$\text{B}_{30}$ operates as a pristine spinless topological semimetal. We show that the combined time-reversal and twofold screw symmetry ($\mathcal{T}S_{2z}$) enforces a robust two-dimensional nodal surface on the $k_z = \pi$ plane via a Kramers-like degeneracy. Concurrently, the system hosts a diverse set of zero-dimensional Weyl fermions -- including an unconventional double-Weyl point ($\mathcal{C} = -2$), conventional Type-I WPs ($\mathcal{C} = -1$), and completely tilted Type-II WPs ($\mathcal{C} = +1$) -- emerging at the high-symmetry points $\Gamma$ and K, as well as along the H-K path, protected by $C_6$ and $C_3$ crystalline rotational symmetries. Crucially, the substantial momentum-space separation between the nodal surface and Weyl points allows for their unambiguous independent resolution. Calculations of the (100) surface states reveal distinct, nontrivial Fermi arcs connecting Weyl nodes of opposite chirality. This work establishes $P6_3$-$\text{B}_{30}$ as a compelling material platform for investigating the physics of multidimensional hybrid topological fermions and their interplay.
Chern insulator systems are realizable in numerous physical systems and can support robust nonreciprocal transmission of energy. A routing functionality constructed from two counter-oriented Chern insulator regions, using coupled Haldane type systems is proposed. By adjusting the strength of a magnetic field and the frequency of an antenna source, it possible to steer the flow of energy: completely to the left, completely to the right, or split. Alternatively, two sources can be used to direct the flow of energy. This formulation has the potential to serve as a robust and reconfigurable component in optical transmission.
Accurate interatomic potentials (IAPs) are essential for modeling the potential energy surfaces (PES) that govern atomic interactions in materials. However, most existing IAPs are developed for bulk materials and often struggle to accurately and efficiently capture the diverse chemical environments of two-dimensional (2D) materials, which limits large-scale simulation and design of emerging 2D systems. To address this challenge, we develop Uni2D, an interatomic potential tailored for 2D materials. The Uni2D model is trained on a dataset comprising approximately 327,000 structure-energy-force-stress mappings derived from about 20,000 distinct 2D materials, covering 89 chemical elements. The model demonstrates reliable predictive performance for energies, forces, and stresses, and demonstrates quantitatively robust accuracy in tasks such as structural relaxation, equation-of-state calculations, and molecular dynamics simulations, making the model suitable for high-throughput screening of 2D materials. For derived properties, including elastic properties, lattice dynamics, and other screening-related metrics, the model provides qualitative to semi-quantitative predictions that remain useful for trend analysis and preliminary evaluation. To enhance usability, we further introduce an intelligent agent powered by a large language model (LLM), enabling automated workflows and natural language interaction for 2D materials simulations. Our work provides an efficient and accessible framework for high-throughput screening and computational exploration of 2D materials.
arXiv:2604.10773v2 Announce Type: replace-cross Abstract: The macroscopic dynamics of topological defects in magnetic materials are traditionally modeled using pairwise interactions. However, higher-order quantum exchange mechanisms - such as biquadratic and 4-spin ring exchange-play a critical role in strongly correlated systems. In this work, we introduce the "Simplicial Bridge," an exact analytical framework that maps these high-dimensional, non-linear Landau-Lifshitz partial differential equations onto generalized Kuramoto phase-oscillator networks operating on abstract simplicial complexes. We rigorously demonstrate that spatial overlap in the continuous limit natively generates higher-order topological forces without requiring a supportive discrete atomic lattice. Specifically, the overlap of 1D helimagnetic kinks generates 2-simplices (triadic forces), while the spatial compression of 2D skyrmion tails - governed by modified Bessel function asymptotics - generates true 3-simplices (tetradic forces). Furthermore, we establish that the higher-order spatial derivatives inherent to these multi-spin interactions provide an intrinsic energetic barrier that bypasses Derrick's Theorem, stabilizing 2D topological solitons without the strict need for Dzyaloshinskii-Moriya Interaction (DMI).
Investigating the interplay among topology and electron-electron interactions is an intriguing research quest which has recently gathered steam across the community of condensed-matter physics. In the present work, we study the fate of a three-dimensional Berry-dipole semimetal, lying at the topological quantum critical point separating a Hopf insulator from a trivial insulator, in the presence of long-range Coulomb interactions. Utilizing large-$N_f$ analysis at three spatial dimensions and an $\epsilon$-expansion within the renormalization-group scheme, we uncover the emergence of a spatially \textit{anisotropic} non-Fermi liquid with enhanced Berry-dipole moment. We further derive the corresponding scaling relations of certain physical observables as functions of the probed energy and temperature scale, and we provide a simple observational criterion for distinguishing the onset of the topological anisotropic non-Fermi liquid from a Berry-dipole semimetal.
Chalcogenide perovskites have emerged as promising lead free materials for photovoltaic and thermoelectric applications. Among them, BaZrS3 has attracted particular attention due to its thermal and chemical stability, favorable optoelectronic properties, and low thermal conductivity. Here, we combine molecular dynamics and Monte Carlo simulations based on machine learned interatomic potentials with scanning transmission electron microscopy to investigate mixing thermodynamics and phase stability in the BaZr(S,Se)3 system. We identify an unusual ordered structure that persists at room temperature, most prominently at 33% S, where S and Se atoms form alternating layers within the crystal. Free energy calculations yield the temperature composition phase diagram, including a nonperovskite delta phase in the Se rich limit and a perovskite phase in the S rich limit, separated by a broad two phase region. Analysis of the dielectric function and the absorption coefficient demonstrates that composition, crystal structure, and anion ordering jointly control the optical band gap. Selenium alloying enables tuning between approximately 1.6 and 1.9eV, while anion ordering within a given composition reduces the gap by about 0.12eV. Lastly, variations between structural polymorphs give rise to band gap differences of up to 0.4eV.
Light-matter interactions are governed by conservation laws of energy and momentum. For harmonic generation in crystalline solids, energy conservation imposes that $m$ incoming photons with energy $\hbar \omega_0$ are combined to form one photon at energy $m\hbar \omega_0$. Linear momentum conservation governs phase matching, whereas angular momentum conservation connects the angular momentum carried by photons to the discrete rotational symmetry of the crystal lattice. As a consequence, circular harmonic generation exerts a torque on the lattice and, conversely, a macroscopic rotation of the crystal induces a nonlinear rotational Doppler shift. These cornerstone laws of nonlinear optics rely on macroscopic symmetry arguments, and therefore provide little insight into the microscopic origin of angular momentum transfer. Here we uncover a direct connection between angular momentum conservation in nonlinear optics and the electronic quantum geometry, by proving that the transferred angular momentum from light to the crystal is proportional to the local Berry curvature at one optical resonance. This relation is encoded in the nonlinear harmonic circular dichroism, which we measure experimentally in an atomically thin semiconductor. With this, we extend our understanding of nonlinear optics, and we establish a method for the all-optical control and read-out of the local Berry curvature.
The nitrogen-vacancy (NV) center in diamond enables optical initialization and readout of its electronic spin, forming the basis of a wide range of quantum sensing and metrology applications. A central challenge in such measurements is the coexistence of two charge states, NV- and NV0: While detection protocols rely on the spin-dependent properties of NV-, fluorescence from NV0 does not carry useful contrast and is typically removed as background, reducing the available signal. Here, we show that the origin of NV0 emission depends strongly on the excitation wavelength in nitrogen-containing diamond. Using ensembles of NV centers with varying nitrogen concentrations, we compare excitation at the NV0 zero-phonon line (ZPL) at 575 nm with the commonly used 532 nm. We find that excitation at 575 nm generates NV0 predominantly through spin-selective tunneling from the excited state of NV- to nearby nitrogen donors, such that the NV0 emission follows the spin polarization of NV-. As a result, the NV0 fluorescence contributes to the measurable spin contrast, allowing the full fluorescence signal to be used for detection. This result opens opportunities for improved sensitivity in NV-based sensing applications.
Symmetry-protected topological phases of matter, characterized by non-trivial band topology, are spectrally gapped and show non-trivial boundary phenomena. Here, we show that scattering states when interjected by an array of periodically modulated defects can result in emergent topological phases whose properties can be tuned by modulating the defect strengths. We dub this the Su-Schrieffer-Heeger network. We show that a scattering-matrix network model can capture the emergent symmetries and nontrivial winding of the quasienergy bands, which lead to distinct transport signatures and can be further periodically driven to realize a robust Thouless charge pump. We show that a microscopic lattice model embedded with a defect superlattice yields Bloch minibands that directly map to the network problem. We further verify that the physics we report is stable to disorder and point out concrete experimental solid-state platforms where it is readily realizable. Our work, in contrast to engineering atomic Hamiltonians, shows that defect engineering on metallic platforms can lead to emergent topological phases of quantum matter.
We investigate the emergence of charge waves and their temporal dynamics in one-dimensional Su-Schrieffer-Heeger (SSH) topological chains. Contrary to the conventional view that charge oscillations are suppressed in gapped topological systems with preserved chiral symmetry, we show that such oscillations can indeed occur. The general condition for an arbitrary oscillation period is analysed, and we find that the charge waves propagating along the chain do not depend on its topology, except at the edges, where both topological phases exhibit essential differences. In chains with inequivalent atoms within the SSH unit cell, we observe regular long-period sublattice oscillations that appear simultaneously with even-odd charge oscillations. Furthermore, we study the nonequilibrium dynamics in SSH chains. After a quench, the time evolution of the local density of states and charge occupancies exhibits clear dynamical fingerprints that distinguish topologically trivial and nontrivial phases. Our results establish that transient charge dynamics can distinguish topologically trivial and nontrivial phases in real time by detecting the presence of topologically-protected edge states.
Coherent control of quantum materials has progressed along two major fronts: nonlinear phononics, which reshapes lattices to induce emergent states, and Floquet engineering, which tailors electronic band reconstruction via time-periodic driving. Both mechanisms face fundamental limitations at terahertz (THz) frequencies: phononic nonlinearities are intrinsically weak in standard lattices, while electronic Floquet states are often constrained by rapid decoherence upon light-off and by a scarcity of coherence-resolved, multi-correlation probes beyond (quasi-)stationary band structures. Here we report an extreme THz nonlinear-phononics mechanism in $\text{Ta}_\text{2}\text{NiSe}_\text{5}$, where a highly susceptible non-equilibrium electronic correlation bath dramatically amplifies lattice nonlinearities under coherent driving. Utilizing THz two-dimensional spectroscopy as a coherence-tomography tool, we resolve an exceptionally rich landscape of approximately 30 distinct multi-order quantum pathways, including high-harmonic phonon generation, multi-quantum coherences, and multi-wave anharmonic cross-mode mixing. The density and complexity of this extreme manifold establishes a new benchmark for THz nonlinear phononics, as the multi-order quantum pathways surpass the limits of conventional lattice responses. These high-order signals collapse above ~100~K, defining an electronic correlation scale of a coherence-imprinted hybrid electronic-phonon order that governs the sustainability of high-order quantum correlations and nonlinear pathways beyond linear and equilibrium responses. Our results establish a route for correlation-boosted, phonon-anchored periodic Hamiltonian engineering and for certifying such periodically-driven states via multi-correlation coherence tomography.
Solid-liquid interfacial thermal conductance (ITC) critically influences heat transport in microfluidic, electronic, and energy systems, yet most optical thermometry techniques are limited to specific metal-liquid interfaces. In this work, we introduce a universal broadband square-pulsed thermometry method that enables simultaneous quantification of ITC across a wide range of arbitrary solid-liquid interfaces, while also providing accurate measurements of nanoscale liquid-film thickness. To validate the method, we applied it to Al-water interfaces, yielding ITC values in the range of 50-55 MW m^(-2) K^(-1), consistent with prior studies. The technique also reveals markedly lower ITCs for glass-water (9.9 MW m^(-2) K^(-1)) and Si-water (5.7 MW m^(-2) K^(-1)), and further measurements on Al-silicone oil (~10 MW m^(-2) K^(-1)) and PMMA-silicone oil (~0.4 MW m^(-2) K^(-1)) extend the validation to highly viscous nonpolar liquids and polymer-liquid interfaces. These results highlight the capability of the method to capture thermal transport differences across diverse solid-liquid combinations. Further comparisons with acoustic/diffuse mismatch models and molecular dynamics simulations, together with theoretical analysis, highlight the influence of vibrational mismatch, wettability, and surface condition on interfacial thermal transport. This broadly applicable technique enables rapid, quantitative characterization of solid-liquid interfacial thermal transport, with broad implications for interfacial heat transfer science and technology.
Many-body effects in condensed matter yield novel quantum states when the electronic density of states is enhanced. A vivid example is flat bands, which suppress kinetic energy and let interactions dominate, when they are filled with an integer number of electrons in moire systems. Yet flat bands and commensurate fillings are not the only conditions for correlated phenomena. Situations may occur where the band structure develops locally enhanced density of states, leading to strong correlations even at non-integer fillings, although such cases often yield pseudogaps that make detection elusive. Here we demonstrate that small-angle twisted monolayer-bilayer graphene combines moire-induced global flat band and additional local band flattening. Their coexistence allows direct comparison of correlated effects. The global route stabilizes commensurate states, while the local mechanism produces nearly flat bands, lifting degeneracy and generating symmetry breaking at non-integer fillings, yet without opening a global gap. Because there is no global gapped signature, the system remains metallic, but the effect reveals itself in anomalous Hall responses, signaling time-reversal symmetry breaking and valley polarization. Our results demonstrate dual-flatness as a guiding principle, extending moire physics beyond commensurate fillings and identifying topological transport as a probe of gapless correlated metals.
We demonstrate that flat-band engineering provides a direct route to control and optimize the thermodynamic performance of quantum heat engines. We consider noninteracting bosons on a rhombi-chain lattice described by a Bose-Hubbard model in the noninteracting limit, where a magnetic flux serves as a tunable parameter that continuously reshapes the single-particle spectrum. By driving the system toward the fully frustrated Aharonov-Bohm caging regime, the band structure transitions from dispersive to completely flat, strongly modifying the thermal occupation of the modes. We show that this flux-induced spectral restructuring has clear and measurable thermodynamic consequences. In particular, the Otto cycle exhibits a significant enhancement of both work output and efficiency when operating near the caging regime. We identify the underlying mechanism as a pronounced suppression of heat released to the cold reservoir, rather than an increase in absorbed heat, revealing that flat-band formation is an effective strategy to increase work extraction. In contrast, the Stirling cycle is governed by entropy variations along isothermal, flux-driven processes, leading to greater work extraction over a broader parameter range but at lower efficiency. These results establish geometric frustration and Aharonov-Bohm caging as thermodynamic resources and show that spectral engineering via synthetic gauge fields offers a viable, experimentally accessible pathway to tailor the performance of bosonic quantum thermal machines.
In a recent work, Somogyfoki et al. (J. Non-Equilib. Thermodyn. 50, 59-76, 2025) analysed the linear stability of homogeneous equilibrium in third-order non-Fourier heat conduction within the framework of non-equilibrium thermodynamics with internal variables. They identified a stability condition, their equation (49), which could not be derived from the standard thermodynamic inequalities for the 2X2 conductivity blocks, and concluded that the Second Law does not guarantee stability in the most general case. Here we show that this conclusion was due to an overly conservative proof strategy: the standard thermodynamic conditions (concave entropy and non-negative entropy production, as expressed by the $2\times2$ block positive-definiteness inequalities (19)-(20) of the original paper) do suffice for linear stability. The key observation is that all coefficients of the dispersion polynomial remain positive for all physical wave numbers because their structure prevents positive real roots. This result confirms that thermodynamics, understood as a stability theory, ensures fundamental dynamic stability in all thermodynamically consistent third-order extended heat conduction theories. A comparison with the rate-equation approach of Giorgi, Morro and Zullo (Meccanica 59, 1757-1776, 2024) is also presented.
Nanoplasmonic modification of scintillation has so far been explored mainly in the weak-coupling regime, where changes in the local density of optical states enhance radiative recombination via Purcell-type rate engineering. By contrast, strong light-matter coupling generates hybrid states that modify emission dynamics beyond simple decay-rate acceleration, but its implications for scintillator nanocrystals (NCs) under ionizing radiation remain poorly understood. All of these effects are beneficial for near-infrared scintillators, which are typically slow and have low brightness. Here, we present a quantum-optical framework to investigate how near-infrared scintillator NCs coupled to nanoplasmonic antennas evolve from weak coupling toward strong light-matter coupling. We compare broad- and narrow-antenna platforms with single and periodic Au nanorods and benchmark them against conductive plasmonic antennas based on indium tin oxide and graphene. As representative emitters, we consider wide-band PbS NCs and narrow-band cubic Lu2O3:Er3+ scintillators. The calculations show that the onset of strong-coupling signatures is jointly governed by emitter dephasing and the antenna linewidth, with narrow-band emitters coupled to spectrally narrow antennas providing the most favorable conditions. Among the platforms considered, graphene gives the lowest threshold (g = 4 meV) for observable coherent exchange owing to its ultranarrow antenna linewidth (\k{appa} = 3.5 meV). These results identify near-infrared conductive nanoantennas, particularly graphene-based ones, as promising platforms for accessing hybrid scintillation regimes relevant to radiation detection.
We predict the emergence of nontrivial topological magnon states in the skyrmionium lattice with zero topological charge. We propose the concept of weighted magnetic flux, which provides a clear physical picture for this anomalous phenomenon. We also map the skyrmionium lattice onto the Haldane model, offering an alternative framework for interpreting this. Our findings challenge the conventional wisdom that such states are linked to nonzero topological charge in skyrmion lattices, offering a new perspective in topological magnonics. To facilitate experimental validation, we propose two methods for preparing the skyrmionium lattice and calculate the induced magnon thermal Hall conductivity, which is a key indicator in transport measurements.
Charge density waves (CDWs) are a widespread collective electronic order in quantum materials, furnishing key insights into symmetry breaking and competing phases. However, their dynamic control with external fields remains a pivotal challenge. Here, we report deterministic and hysteretic switching of unidirectional CDW orientation via in-plane magnetic field rotation in magnetic kagome metal GdTi3Bi4. Atomically resolved spectroscopy shows two types of 3a0*1a0 CDW domains, Q1 and Q2 oriented 60 degree apart along two distinct crystallographic directions and separated by atomically sharp domain walls. Rotating the magnetic field drives reversible transitions between these CDW configurations, exhibiting a robust C2-symmetric phase diagram with pronounced hysteresis. This hysteretic switching is mediated by a field-dependent reorientation of underlying antiferromagnetic spins, revealing a tunable energy landscape with stable and metastable states and modulates the electronic charge order via spin-lattice coupling. Our findings not only demonstrate the switching of CDW configurations by in-plane magnetic field but also reveal the mechanism of coupling between CDW and magnetic fields, offering new insights into CDW manipulation and versatile platform for developing a spin-mediated multistate spin-charge coupling memory and programmable quantum devices.
This study presents a 3D version of multiscale approach for investigating magnetization dynamics in multiscale, hybrid micromagnetic-atomistic simulations. The present work introduces engineered discontinuities (i) a double-slit structure, which enables the study of domain wall and spin wave interference, and (ii) a tetrahedron shaped cluster of atoms with tunable anisotropy, which provides insights into how localized anisotropic perturbations influence domain wall pinning and skyrmion stability in fully three-dimensional (3D) hybrid simulations. We considered the dynamics of spin waves, domain walls, as well as 3D skyrmions, in the presence of these defects. The magnonic double-slit experiment demonstrates interference patterns analogous to electronic wave phenomena, offering potential applications in wave-based computing. Additionally, the results reveal the impact of the local anisotropy that leads to distinct transformations, including domain wall deformations, tubular and spherical structures, skyrmion annihilation, and breathing mode. The findings underscore the critical role of defect-induced anisotropic interactions in controlling domain wall motion, skyrmion topology, and spin wave propagation.
We have performed detailed temperature-dependent study of optical f-f transitions of the Yb3+ ions in h-YbMnO3 by means of Fourier-transform spectroscopy. The splitting of the ground Kramers doublet as a function of temperature, D0(T), for the Yb3+ ion at 4b site was determined. The D0(T) function follows the dynamics of the manganese magnetic moment below TN = 87 K, indicating, that the ytterbium subsystem is magnetized by the magnetic field generated by an ordered manganese subsystem, which is consistent with the results of previous studies. Excitation of the upper component of the split ground doublet plays a significant role in low-temperature dynamics of the h-YbMnO3 crystal. Using the D0(T) function we calculated the temperature behavior of the of the Yb(4b) magnetic moment: it is in clear agreement with the neutron data [Phys. Rev. B 98, 134413, 2018]. The calculated contribution of Yb(4b) to heat capacity definitely explains the origin of the Schottky anomaly in the CP(T) dependence. A scenario for phase transitions in h-YbMnO3 is proposed in which the energy gain in the ytterbium system plays a key role.
We introduce the subdimensional entanglement entropy (SEE), defined on subdimensional entanglement subsystems (SESs) embedded in the bulk, as an entanglement-based probe of how geometry and topology jointly shape universal properties of quantum matter. By varying the dimension, geometry, and topology of the SES, we show that the subleading term of SEE exhibits sharply distinct responses in different phases, including cluster states, $\mathbb{Z}_q$ topological orders, and fracton orders. Treating the reduced density matrix of an SES as a many-body mixed state supported on the SES manifold, we further establish a general correspondence between bulk stabilizers and mixed-state symmetries on SESs, separating them into strong and weak classes, and use it to identify strong-to-weak spontaneous symmetry breaking within SESs. Finally, for SESs with nontrivial SEE, we show that weak symmetries act as transparent patch operators of the corresponding strong symmetries. This motivates the notion of transparent composite symmetry, which remains robust under finite-depth quantum circuits that preserve SEE, and implies that each $D$-dimensional SES holographically encodes a $(D+1)$-dimensional topological order. These results establish SEE not only as a sharp probe of geometric-topological response, but also as a route from bulk pure-state entanglement to mixed-state symmetry and holography on subdimensional manifolds.
We study a Su-Schrieffer-Heeger chain coupled to a single mode photonic cavity. Considering an off-resonant regime we use the high-frequency expansion in order to obtain an effective fermionic Hamiltonian with cavity-mediated interactions. We characterize the effects of the cavity on topology in a finite size chain by studying three different markers adapted for interacting systems: correlation functions between edges in a chain with open boundary conditions, and a winding number based on the single-particle Green's function and bulk electric polarization via the many-body formula by Resta for a chain with periodic boundary conditions. There is excellent agreement between the winding number and polarization approaches to compute the phase diagram, with the presence of the edge states being confirmed through the calculations of the two-point correlation function. Our approach provides an alternative perspective on cavity-modified topological phases through a study of an effective interacting electronic Hamiltonian and complements methods that treat the full light-matter Hamiltonian directly.
Aluminum nitride (AlN)-based thin-film bulk acoustic wave resonators (FBARs) are promising compact platforms for 6G communications and quantum memory hardware, enabled by their integrable acoustic modes with high quality factors. However, temperature-dependent acoustic dissipation ultimately limits device performance. In this work, we fabricated a 16 GHz epitaxial AlN FBAR as a test platform, performed small-signal RF measurements from 6.5 K to 300 K, and developed a physics-based model to estimate the fundamental quality-factor limits of FBARs to cryogenic temperatures. The proposed model incorporates both intrinsic and extrinsic loss mechanisms, including an analytical anchor-radiation loss model for bulk acoustic wave resonators, rather than relying solely on finite-element simulations. Measured loaded quality factor (Q) decreases monotonically with temperature, from Qmax of approximately 1589 (Qf=24.79 THz) at 6.5 K to 363 at 294K (Qf=5.66 THz). This trend is consistent with the theoretical limit based on the resonator geometry and the chosen Metal-Insulator-Metal (MIM) stack. To demonstrate the generality of the physics-based framework, we further validate it by benchmarking against a 23 GHz high-overtone bulk acoustic resonator (HBAR) using previously reported data. The validated model provides a practical, transferable framework to interpret Q(T) limits in low-loss resonators by quantifying the temperature-dependent mechanisms that constrain Q, enabling the design of cryogenic microwave filter elements for superconducting quantum hardware.
Spin qubits have emerged as a leading platform for quantum information processing due to their long coherence times, small footprint, and compatibility with the existing semiconductor industry. We first provide an introduction to the different qubit implementations currently being investigated, including single electron-spin qubits, hole-spin qubits, donor qubits, and multispin encodings. We discuss how the confinement and strain present in semiconductor heterostructures produce addressable levels whose spin degree of freedom can be used to encode a qubit. A large emphasis is placed on reviewing the theoretical foundations and recent experimental demonstrations of proposed mechanisms for long-range coupling, including hybrid approaches based on circuit QED and Andreev qubits, as well as spin shuttling. Finally, we review a recent proposal for linking spin qubits using topological spin textures.
Scientific Reports, Published online: 15 April 2026; doi:10.1038/s41598-026-48902-8
ADAM15 promotes the progression and metastasis of hepatocellular carcinoma by activating the JNK/p38 pathwayDistinguishing different subphases in the supercritical region is a fundamental issue in statistical physics and condensed matter physics. Traditional approaches mainly rely on static thermodynamic response functions or equilibrium correlation functions, which are inherently confined to quasi-static processes. In this work, we adopt a nonequilibrium dynamical perspective to investigate the evolution of a holographic superfluid model following a rapid quench across the critical point. We find that the invasion phenomenon induced by topological defects persists in the supercritical region, and the invasion velocity exhibits a clear turning point as a function of the quench endpoint $\rho_f$. This turning point defines a new nonequilibrium supercritical crossover line. In contrast to the classical Widom line or Frenkel line, this new crossover line encodes both thermodynamic information and kinetic information, reflecting the dynamical nature of the supercritical region under nonequilibrium conditions. This study provides a novel nonequilibrium dynamical approach for characterizing supercritical subphases.
We study $\mathbb{Z}_3$-symmetric Rabi model that describes a three-level system coupled to two bosonic modes. We derive a mapping of the two-mode $\mathbb{Z}_3$ Rabi model onto a qubit-boson ring. This mapping allows us to formulate a realistic implementation of the $\mathbb{Z}_3$ Rabi model based on superconducting qubits. It also provides context for the previously proposed optomechanical implementation of the $\mathbb{Z}_3$ Rabi model. In addition, we propose a physical implementation of the $\mathbb{Z}_3$ Potts model via a coupled chain of $\mathbb{Z}_3$ Rabi models.
Time-resolved scanning near-field optical microscopy (tr-SNOM) enables the measurement of the dynamic optical response of functional surfaces beyond the diffraction limit. Experimental challenges are imposed both by the use of a pulsed light source, and by the need for interferometric signal modulation to isolate the near-field contribution. We present a novel experimental approach to retrieve the tr-SNOM signal using a 200 kHz laser system and pseudo-heterodyne modulation. We circumvent the Nyquist limit for spectral demodulation by sampling modulation phases, pump intensity and SNOM signal for every laser shot. A general time-resolved SNOM signal is derived, independent of detection scheme or physical assumptions about the near-field enhancement, and is successfully measured and isolated on WS$_2$ monolayer and multilayer regions. We confirm localization by signal-distance curves, spatial confinement at material boundaries, and by identifying signal contributions at individual modulation harmonics. Disentangling the dynamic contributions enables us to extract the dynamic dielectric function of the sample. Showing the capability of phase-domain sampling paves the way to integration of more diverse and specialized light sources, growing the potential of optical ultrafast near-field measurements.
Advanced Science, EarlyView.
If an operator $H$ anticommutes with a chirality operator $\Gamma_*$ such that $\Gamma_*^2=1$, the null space of $H$ can be decomposed in a direct sum of two spaces having positive and negative chiralities, respectively. When both spaces are finite dimensional, one can define an index, $\mathrm{Ind}(\Gamma_*,H)$, as the difference of dimensions of these two spaces. The key issue is whether $\mathrm{Ind}(\Gamma_*,H)$ is topologically protected, i.e., whether it remains constant under smooth variations of the parameters and background fields entering $H$. For Hermitian Dirac operators, topological protection of the index is guaranteed by the Atiyah--Singer theorem. In this paper, by using the heat kernel methods, we show that $\mathrm{Ind}(\Gamma_*,H)$ is topologically protected also for non-hermitian operators $H$ as long as they are diagonalizable and satisfy some ellipticity conditions.
In many real-world problems, recovering sparse signals from underdetermined linear systems remains a fundamental challenge. Although $\ell_1$ norm minimization is widely used, it suffers from estimation bias that prevents it from reaching the Bayes-optimal reconstruction limit. Nonconvex alternatives, such as the log-sum penalty, have been proposed to promote stronger sparsity. However, maintaining their algorithmic stability is challenging. To address this challenge, we introduce an adaptive smoothing strategy within an approximate message passing framework to mitigate algorithmic instability. Furthermore, we evaluate the typical exact-recovery threshold for Gaussian measurement matrices using the replica method and state evolution. The results indicate that the adaptive method achieves exact recovery over a broader region than $\ell_1$ norm minimization, although metastable states hinder reaching the information-theoretic limit.
Advanced Science, EarlyView.